The Role of the Eu3+ Concentration on the SrMoO4:Eu Phosphor Properties: Synthesis, Characterization and Photophysical Studies View Full Text


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Article Info

DATE

2011-05

AUTHORS

Ana Paula A. Marques, Marcos Takashi S. Tanaka, Elson Longo, Edson R. Leite, Ieda Lucia Viana Rosa

ABSTRACT

SrMoO(4) doped with rare earth are still scarce nowadays and have attracted great attention due to their applications as scintillating materials in electro-optical like solid-state lasers and optical fibers, for instance. In this work Sr(1-x)Eu(x)MoO(4) powders, where x=0.01; 0.03 and 0.05, were synthesized by Complex Polymerization (CP) Method. The structural and optical properties of the SrMoO(4):Eu(3+) were analyzed by powder X-ray diffraction patterns, Fourier Transform Infra-Red (FTIR), Raman Spectroscopy, and through Photoluminescent Measurements (PL). Only a crystalline scheelite-type phase was obtained when the powders were heat-treated at 800 °C for 2 h, 2θ=27.8° (100% peak). The excitation spectra of the SrMoO(4):Eu(3+) (λ(Em.)=614 nm) presented the characteristic band of the Eu(3+5)L(6) transition at 394 nm and a broad band at around 288 nm ascribed to the charge-transfer from the O (2p) state to the Mo (4d) one in the SrMoO(4) matrix. The emission spectra of the SrMoO(4):Eu(3+) powders (λ(Exc.)=394 and 288 nm) show the group of sharp emission bands among 523-554 nm and 578-699 nm, assigned to the (5)D(1)→(7)F(0,1 and 2) and (5)D(0)→(7)F(0,1,2,3 and 4), respectively. The band related to the (5)D(0)→(7)F(0) transition indicates the presence of Eu(3+) site without inversion center. This hypothesis is strengthened by the fact that the band referent to the (5)D(0)→(7)F(2) transition is the most intense in the emission spectra. More... »

PAGES

893-899

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10895-010-0604-6

DOI

http://dx.doi.org/10.1007/s10895-010-0604-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1028602098

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/20177748


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