Synthesis and characterization of (Cu1−xAgx)2ZnSnS4 nanoparticles with phase transition and bandgap tuning View Full Text


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Article Info

DATE

2020-03-09

AUTHORS

Ning Liu, Fei Xu, Yan Zhu, Yongmao Hu, Guitang Liu, Liang Wu, Kangjing Wu, Shuhong Sun, Feng Hong

ABSTRACT

Multi-component chalcogenide (Cu1−xAgx)2ZnSnS4 (CAZTS, x = 0, 0.1, 0.2, 0.3, 0.4) nanoparticles were synthesized by incorporation of Ag into wurtzite Cu2ZnSnS4 (CZTS) using a simple one-pot method and were characterized by X-ray diffraction, Raman spectroscopy, transmission electron microscopy, scanning electron microscopy, X-ray photoelectron spectroscopy, and UV–Vis–NIR absorption spectrum, respectively. The synthesized nanoparticles exhibit the phase transition from wurtzite to kesterite structure when the substitution ratio (x) of Ag is around 0.3. The bandgaps of CAZTS nanoparticles are in the range of 1.43–1.64 eV. This finding indicates that Ag substitution in wurtzite CZTS is an effective way to adjust the bandgap and structure. More... »

PAGES

5760-5768

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10854-020-03146-8

DOI

http://dx.doi.org/10.1007/s10854-020-03146-8

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1125505832


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