Construction and characterization of BiOI/NH2-MIL-125(Ti) heterostructures with excellent visible-light photocatalytic activity View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2019-02

AUTHORS

Li Han, Xiaomin Zhang, Deyong Wu

ABSTRACT

To utilize the synergistic effect between BiOI and NH2-MIL-125(Ti), a series of BiOI/NH2-MIL-125(Ti) heterostructures with different NH2-MIL-125(Ti) contents were fabricated. The characterization of BiOI/NH2-MIL-125(Ti) was performed by XRD, SEM, TEM, FT-IR, XPS and DRS. The results showed that NH2-MIL-125(Ti) catalysts were highly dispersed on the surface of BiOI nanosheets. Compared to pure BiOI and NH2-MIL-125(Ti) photocatalyst, BiOI/NH2-MIL-125(Ti) composites displayed superior visible light photocatalytic activity. The enhanced photocatalytic performance was ascribed to the formation of heterojunction structure between BiOI nanosheets and NH2-MIL-125(Ti), which significantly suppressed the recombination of photogenerated electron–hole pairs. The optimal content of NH2-MIL-125(Ti) was about 7 wt%, and photocatalytic degradation rate was about 3.8 times and 12.2 times of BiOI and NH2-MIL-125(Ti), respectively. In addition, BiOI/NH2-MIL-125(Ti) composites could keep the photocatalytic activity during the cycle experiment. More... »

PAGES

3773-3781

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10854-018-00660-8

DOI

http://dx.doi.org/10.1007/s10854-018-00660-8

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1111057988


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61 schema:description To utilize the synergistic effect between BiOI and NH2-MIL-125(Ti), a series of BiOI/NH2-MIL-125(Ti) heterostructures with different NH2-MIL-125(Ti) contents were fabricated. The characterization of BiOI/NH2-MIL-125(Ti) was performed by XRD, SEM, TEM, FT-IR, XPS and DRS. The results showed that NH2-MIL-125(Ti) catalysts were highly dispersed on the surface of BiOI nanosheets. Compared to pure BiOI and NH2-MIL-125(Ti) photocatalyst, BiOI/NH2-MIL-125(Ti) composites displayed superior visible light photocatalytic activity. The enhanced photocatalytic performance was ascribed to the formation of heterojunction structure between BiOI nanosheets and NH2-MIL-125(Ti), which significantly suppressed the recombination of photogenerated electron–hole pairs. The optimal content of NH2-MIL-125(Ti) was about 7 wt%, and photocatalytic degradation rate was about 3.8 times and 12.2 times of BiOI and NH2-MIL-125(Ti), respectively. In addition, BiOI/NH2-MIL-125(Ti) composites could keep the photocatalytic activity during the cycle experiment.
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