Effects of donor position on dibenzofulvene-based organic dyes for photovoltaics View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2017-06

AUTHORS

Giuseppina Anna Corrente, Eduardo Fabiano, Luisa De Marco, Gianluca Accorsi, Roberto Giannuzzi, Antonio Cardone, Giuseppe Gigli, Giuseppe Ciccarella, Agostina-Lina Capodilupo

ABSTRACT

A series of push–pull organic dyes based on the cyanoacrylic acid as the acceptor/anchoring group, a dibenzofulvene (DBF) connected with thienyl rings as the π-bridge, and donor units linked to different positions of the DBF molecule were synthetized and studied. The effects of the donor position on optical and photovoltaic properties were investigated through photophysics, electrochemical and photovoltaic measurements. The results uphold photovoltaic performances largely depend on the electronic structure of the dyes with a synergistic interaction between donor and acceptor groups. In detail, a fine tuning of the photophysical properties can be reached simply selecting the position of the donor unit on the DBF molecule. In particular, the dyes bearing the donor unit on the 3,6-positions of the DBF show better performances in term of light absorption and cell efficiency with respect to the dyes with the donor unit on the 2,7-positions. More... »

PAGES

8694-8707

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10854-017-6594-2

DOI

http://dx.doi.org/10.1007/s10854-017-6594-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1084027425


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