Solute adsorption and exclusion studies of the structure of never-dried and re-wetted cellulosic fibres View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2007-08

AUTHORS

R. N. Ibbett, S. Kaenthong, D. A. S. Phillips, M. A. Wilding

ABSTRACT

The total water capacity of a series of never-dried and re-wetted cellulosic fibres has been shown to correlate with the accessible volume described by a thermodynamic model. The model was applied to interpret the adsorption behaviour of a range of reactive dyes in electrolyte solutions and was successful in accounting for differences in fibre anionic charge. Comparative solute exclusion data indicated the existence of a population of very small spaces in never-dried cellulosic fibres, which may be associated with water disrupting the cellulose \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${1\overline{1}0}$$\end{document} crystal planes. Such intra-crystalline spaces may provide sites for uptake of planar substantive dyes and may also be accessible to sodium ions. The study showed that never-dried lyocell undergoes a large reduction in total wet capacity following initial drying, which is believed to be due to both exudation of crystal water and to inter-fibrillar crystallisation. This crystallisation mechanism may not be so effective for viscose and modal, which have poorer structural organization. Re-wetted lyocell exhibits high dye adsorption, which may result from the development of a uniform fibrillar morphology with a high surface area. This structural aspect is not expressed by the thermodynamic model. More... »

PAGES

6809-6818

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10853-006-1426-4

DOI

http://dx.doi.org/10.1007/s10853-006-1426-4

DIMENSIONS

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