Fabrication of Magnéli phase Ti4O7 nanorods as a functional sulfur material host for lithium-sulfur battery cathode View Full Text


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Article Info

DATE

2020-03-26

AUTHORS

Shanshan Yao, Ruiduo Guo, Zongzhen Wu, Mingquan Liu, Xinye Qian, Xiangqian Shen, Tianbao Li, Li Wang, Yanhua Wang, Shibiao Qin

ABSTRACT

In this paper, we report a facile approach to synthesize pure Magnéli phase Ti4O7 nanostructures via solvothermal processing and subsequent thermal treatment. The one-dimensional nanostructure of Ti4O7 nanorods (1D Ti4O7 NRs) was characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM) and high-resolution transmission electron microscopy (HRTEM). The as-obtained Ti4O7 NRs, with an average diameter of 150 nm, were used as sulfur host to prepare Ti4O7 NRs/sulfur cathode for lithium-sulfur (Li-S) batteries. Electrochemical measurements showed that the as-synthesized Ti4O7 NRs can improve the electrochemical reaction kinetics during the charge-discharge processes. The initial discharge capacity of the Ti4O7 NRs/sulfur cathode was 930 mAh g−1, and the remaining capacity was 490 mAh g−1 after 500 cycles at 1C, much higher than that of acetylene black/sulfur cathode. Electrochemical impedance spectroscopy (EIS) demonstrated Ti4O7 NRs/sulfur decreases the charge transfer resistance. Moreover, Ti4O7 NRs/sulfur composite exhibits low electrode polarization accompanied by a high lithium ion diffusion coefficient. More... »

PAGES

154-162

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10832-020-00206-7

DOI

http://dx.doi.org/10.1007/s10832-020-00206-7

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https://app.dimensions.ai/details/publication/pub.1125904120


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