Co-sensitized TiO2 electrodes with different quantum dots for enhanced hydrogen evolution in photoelectrochemical cells View Full Text


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Article Info

DATE

2019-03-06

AUTHORS

Andrea Cerdán-Pasarán, Tzarara López-Luke, Isaac Zarazúa, Elder De la Rosa, Rosalba Fuentes-Ramírez, K. C. Sanal, Alejandro Alatorre-Ordaz

ABSTRACT

A comparative study of hydrogen evolution in devices based on cadmium chalcogenides quantum dots (CdS, CdSe and CdTe) and its combinations, sensitizing TiO2 was carried out. A maximum photocurrent of 2.7 mA cm−2 at 0 V bias, and a solar-to-hydrogen (STH) conversion efficiency of 0.9%, was obtained with CdSe QDs due to its wide absorption range. The co-sensitized device with CdS–CdSe QDs showed a higher photocurrent of 3.9 mA cm−2 with an STH of 1.2%. The improvement in hydrogen generation for electrodes sensitized with CdS in combination with CdSe or CdTe QDs, was attributed to the increased light absorption and appropriate band alignment for the enhanced charge transport.Graphical abstract More... »

PAGES

475-484

References to SciGraph publications

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  • 2009-06. An essay on synthetic chemistry of colloidal nanocrystals in NANO RESEARCH
  • 2016-05-14. Photovoltaic study of quantum dot-sensitized TiO2/CdS/ZnS solar cell with P3HT or P3OT added in JOURNAL OF APPLIED ELECTROCHEMISTRY
  • 2016-06-11. The effect of number of SILAR cycles on morphological, optical and photo catalytic properties of cadmium sulfide–titania films in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
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    http://scigraph.springernature.com/pub.10.1007/s10800-019-01299-x

    DOI

    http://dx.doi.org/10.1007/s10800-019-01299-x

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