Towards a new definition of EPOC parameters for anionic electrochemical catalysts: case of propene combustion View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2008-03-20

AUTHORS

Reda Karoum, Antonio de Lucas-Consuegra, Fernando Dorado, Jose Luis Valverde, Alain Billard, Philippe Vernoux

ABSTRACT

The electrochemical promotion of catalysis (EPOC) of propene combustion was investigated using Pt sputtered thin film on an O2− conductor, 8 mol% Y2O3-stabilized-ZrO2 (YSZ). In order to separate the influence of the thermal migration of the O2− oxide ions from the electrolyte to the catalyst surface and the impact of an electrical polarization on the catalytic activity, several light-off experiments (cool down and heat up procedures) were successively performed under different polarizations, i.e. OCV, +2 and −2 V. These experiments have clearly shown that the presence of O2− (thermally or electrochemically induced) inhibits the catalytic activity of the platinum for the propene deep oxidation. These results demonstrate the importance to define a normalized rate enhancement ratio, ρn, from a reference value of the catalytic rate corresponding to a Pt surface state free of O2− ions. More... »

PAGES

1083-1088

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10800-008-9538-y

DOI

http://dx.doi.org/10.1007/s10800-008-9538-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1004744079


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