Effect of silica-nanoparticle fillers on the Johari-Goldstein-β process in polymer nanocomposites View Full Text


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Article Info

DATE

2021-12-13

AUTHORS

Makina Saito, Ryo Mashita, Toshiji Kanaya, Hiroyuki Kishimoto, Yoshitaka Yoda, Makoto Seto

ABSTRACT

The Johari-Goldstein-(JG)-β process dominates some of the mechanical properties of polymeric systems. We studied the JG-β dynamics in a rubber nanocomposite, which is a model system of tire rubber, by quasi-elastic scattering experiments using time-domain interferometry. We observed that the time scale of the local motion of the polymer chain started to decouple from the time scale of the chain diffusion motion on cooling in deeply supercooled region. The temperature dependence of the local relaxation time follows the Arrhenius law down to the glass transition temperature. The JG-β process dominates the local polymer dynamics in the polymer nanocomposite system around the glass transition temperature, similar to the case of the neat polybutadiene system. The time scale of the JG-β process in the polymer nanocomposite system was two times longer than that of the neat polybutadiene system. These results suggest that the presence of silica nanoparticles slows down JG-β relaxations and provides a new clue for understanding the mechanical relaxation properties of polymeric products from a microscopic viewpoint. More... »

PAGES

58

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URI

http://scigraph.springernature.com/pub.10.1007/s10751-021-01784-w

DOI

http://dx.doi.org/10.1007/s10751-021-01784-w

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https://app.dimensions.ai/details/publication/pub.1143840747


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195 schema:name Japan Synchrotron Radiation Research Institute, 679-5198, Sayo, Hyogo, Japan
196 rdf:type schema:Organization
197 grid-institutes:grid.69566.3a schema:alternateName Department of Physics, Tohoku University, 980-8578, Sendai, Miyagi, Japan
198 schema:name Department of Physics, Tohoku University, 980-8578, Sendai, Miyagi, Japan
199 Institute for Integrated Radiation and Nuclear Science, Kyoto University, 590-0494, Kumatori, Osaka, Japan
200 rdf:type schema:Organization
 




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