Emission Mössbauer spectroscopy study of fluence dependence of paramagnetic relaxation in Mn/Fe implanted ZnO View Full Text


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Article Info

DATE

2016-12

AUTHORS

H. Masenda, S. Geburt, K. Bharuth-Ram, D. Naidoo, H. P. Gunnlaugsson, K. Johnston, R. Mantovan, T. E. Mølholt, M. Ncube, S. Shayestehaminzadeh, H. P. Gislason, G. Langouche, S. Ólafsson, C. Ronning, ISOLDE Collaboration

ABSTRACT

Emission Mössbauer Spectroscopy following the implantation of radioactive precursor isotope 57Mn+ (T1/2= 1.5 min) into ZnO single crystals at ISOLDE/CERN shows that a large fraction of 57Fe atoms produced in the 57Mn beta decay is created as paramagnetic Fe3+ with relatively long spin-lattice relaxation times. Here we report on ZnO pre-implanted with 56Fe to fluences of 2×1013, 5×10 13 and 8 × 1013 ions/cm2 in order to investigate the dependence of the paramagnetic relaxation rate of Fe3+ on fluence. The spectra are dominated by magnetic features displaying paramagnetic relaxation effects. The extracted spin-lattice relaxation rates show a slight increase with increasing ion fluence at corresponding temperatures and the area fraction of Fe3+ at room temperature reaches a maximum contribution of 80(3)% in the studied fluence range. More... »

PAGES

40

References to SciGraph publications

  • 2010-04. Observation of spin-lattice relaxations of dilute Fe3+ in MgO by Mössbauer spectroscopy in HYPERFINE INTERACTIONS
  • 2010-12. A ten-year perspective on dilute magnetic semiconductors and oxides in NATURE MATERIALS
  • 2013-05. Stability of the Fe3 + state in ZnO in HYPERFINE INTERACTIONS
  • 2005-09. Ferromagnetism of ZnO and GaN: A Review in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
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    http://scigraph.springernature.com/pub.10.1007/s10751-016-1293-6

    DOI

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