A Composite Catalyst with a Lamellar Fe3O4/Pt/Fe3O4 Structure and Complementary Dual Catalytic Functions View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2015-07

AUTHORS

Satoshi Kameoka, Satoru Wakabayashi, Kazuki Ohshima, An Pang Tsai

ABSTRACT

A composite catalyst with a lamellar Fe3O4/Pt/Fe3O4 structure has been prepared from an Al67Pt7Fe26 (at.%) alloy by leaching with an aqueous 10 % NaOH solution. The lamellar Fe3O4/Pt/Fe3O4 phase exhibits significant catalytic performance as measured by activity and selectivity during the steam reforming of methanol SRM:CH3OH+H2O→CO2+3H2 superior to the catalytic performance of Pt obtained from Al2Pt and a conventional impregnated Pt/Fe3O4 catalyst under the same reaction conditions. It is clear that the Pt and Fe3O4 were primarily responsible for the catalysis of the decomposition of methanol DM:CH3OH→CO+2H2 and the water gas shift reaction WGSR:CO+H2O⇄CO2+H2, respectively. These two reactions work together in a complementary manner to facilitate the overall SRM reaction due to efficient the heat transfer characteristics of the lamellar Fe3O4/Pt/Fe3O4 structure. In this study, we demonstrate that a lamellar structure is available to couple two separate reactions to obtain a new catalytic function. In order to improve catalytic properties (stability, functionality), we combined with eutectic alloys and leaching treatment to obtain alternately binary phases with nano-architecture for catalytic materials. More... »

PAGES

1457-1463

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10562-015-1553-0

DOI

http://dx.doi.org/10.1007/s10562-015-1553-0

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1030091098


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