Preparation of Nano-Composited Catalyst from the Bulk Intermetallic Compound AuZr3 with Hydrogen Absorption View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2010-10

AUTHORS

Naruki Endo, Satoshi Kameoka, An Pang Tsai, Toshiya Hirata, Chikashi Nishimura

ABSTRACT

Calcination-induced catalytic activity of CO oxidation reaction (CO + 1/2O2 → CO2) for an intermetallic, AuZr3 and a hydride, AuZr3Hx (x = 4.8) has been studied. The catalytic activities for both samples were originated from the formation of nano-gold particles and nano-crystalline ZrO2, result by oxidation upon calcination. Oxidation of the AuZr3Hx occurred at lower temperature than the AuZr3, gave rise to the formation of more homogenous distribution and smaller sizes of nano-gold particles (~5 nm) on ZrO2, which were responsible for relatively high catalytic performance. This study provides the possibility of hydrogen absorption treatment being a beneficial process for obtaining nano-composite from intermetallic compounds for catalysts. Oxidation of the hydrogen absorbed AuZr3Hx (x = 4.8) occurred at much lower temperature than that of the AuZr3. The calcined AuZr3Hx exhibited more homogenous distribution of nano-gold particles with smaller sizes (~5 nm) on the ZrO2, which were responsible for relatively high performance of CO oxidation. More... »

PAGES

67-71

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10562-010-0397-x

DOI

http://dx.doi.org/10.1007/s10562-010-0397-x

DIMENSIONS

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131 National Institute for Materials Science (NIMS), 305-0003, Tsukuba, Japan
132 rdf:type schema:Organization
133 https://www.grid.ac/institutes/grid.69566.3a schema:alternateName Tohoku University
134 schema:name Department of Materials Processing, Graduate School of Engineering, Tohoku University, Aoba-yama 6-6-02, 980-8579, Sendai, Japan
135 Institute of Multidisciplinary Research for Advanced Materials (IMRAM), Tohoku University, 2-1-1 Katahira, Aoba-ku, 980-8577, Sendai, Japan
136 rdf:type schema:Organization
 




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