Solvation and Rotational Diffusion of Solutes in Room Temperature Ionic Liquids as Studied by EPR Spectroscopy with Nitroxide Spin Probing ... View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-08

AUTHORS

Yusuke Miyake, Akio Kawai

ABSTRACT

In this article, we briefly introduced our studies on solvation and rotational diffusion of solutes in room temperature ionic liquids (RTILs) by electron paramagnetic resonance with nitroxide spin probing method. Most of the rotational correlation times for the nitroxide radicals are within the range calculated on the basis of Stokes–Einstein–Debye hydrodynamic theory with stick and slip boundary conditions or Gierer–Wirtz theory except for smaller solutes in some RTILs with smaller BF4 and PF6 anions. In RTILs with 1-butyl-3-methylimidazolium as cation and BF4 or PF6 as anion, nitroxide radicals undergo rotational diffusion like supercooled liquids and nitroxide radical with smaller volume rotationally slips. More... »

PAGES

825-835

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00723-018-1025-y

DOI

http://dx.doi.org/10.1007/s00723-018-1025-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1104560833


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