Synthesis of a conjugated pyrrolopyridazinedione–benzodithiophene (PPD–BDT) copolymer and its application in organic and hybrid solar cells View Full Text


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Article Info

DATE

2017-05

AUTHORS

Astrid-Caroline Knall, Andrew O. F. Jones, Birgit Kunert, Roland Resel, David Reishofer, Peter W. Zach, Mindaugas Kirkus, Iain McCulloch, Thomas Rath

ABSTRACT

ABSTRACT: Herein, we describe the synthesis and characterization of a conjugated donor-acceptor copolymer consisting of a pyrrolopyridazinedione (PPD) acceptor unit, and a benzodithiophene (BDT) donor unit. The polymerization was done via a Stille cross-coupling polycondensation. The resulting PPD-BDT copolymer revealed an optical bandgap of 1.8 eV and good processability from chlorobenzene solutions. In an organic solar cell in combination with PC70BM, the polymer led to a power conversion efficiency of 4.5%. Moreover, the performance of the copolymer was evaluated in polymer/nanocrystal hybrid solar cells using non-toxic CuInS2 nanocrystals as inorganic phase, which were prepared from precursors directly in the polymer matrix without using additional capping ligands. The PPD-BDT/CuInS2 hybrid solar cells showed comparably high photovoltages and a power conversion efficiency of 2.2%. GRAPHICAL ABSTRACT: More... »

PAGES

855-862

References to SciGraph publications

  • 2015-03. Status of the crystallography beamlines at Elettra in THE EUROPEAN PHYSICAL JOURNAL PLUS
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    http://scigraph.springernature.com/pub.10.1007/s00706-017-1949-1

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    http://dx.doi.org/10.1007/s00706-017-1949-1

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    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/28458400


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