Ontology type: schema:ScholarlyArticle
1997-12
AUTHORSTh. Freudenberg, W. Radloff, H.-H. Ritze, V. Stert, F. Noack, I.V. Hertel
ABSTRACTThe dynamics of ammonia clusters excited to the à state with 160 fs laser pulses of 6.2 eV was studied by pump-probe experiments with a low probe photon energy of 3.1 eV. Protonated as well as unprotonated cluster ion signals have been observed. The time evolution of both species is characteristic of the intermediate rearrangement and fragmentation processes. The observations strongly support a previously developed kinetic model for this dynamics with the signal at long delay times>6 ps reflecting the species involved in the absorption dissociation ionization (ADI) mechanism. Strong evidence is found for the formation of an internally ‘quasi protonated’ excited state and of ammoniated NH4 radicals. More... »
PAGES267-273
http://scigraph.springernature.com/pub.10.1007/s004600050322
DOIhttp://dx.doi.org/10.1007/s004600050322
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