Ferric/ferrous ratio in silicate melts: a new model for 1 atm data with special emphasis on the effects of melt ... View Full Text


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Article Info

DATE

2018-12

AUTHORS

Alexander Borisov, Harald Behrens, Francois Holtz

ABSTRACT

The effect of MgO and total FeO on ferric/ferrous ratio in model multicomponent silicate melts was investigated experimentally in the temperature range 1300–1500 °C at 1 atm total pressure in air. We demonstrate that the addition of these weak network modifier cations results in an increase of Fe3+/Fe2+ ratio in both mafic and silicic melts. Based on present and published experimental data, a new empirical equation is proposed to predict the ferric/ferrous ratio as a function of oxygen fugacity, temperature and melt composition. In contrast to previous equations, the compositional effect of melts on the Fe3+/Fe2+ ratio is not only modeled by the sum of the molar fraction of the individual oxide components. Additional interactions terms have also been incorporated. The main advantage of the proposed model is its applicability for a wide compositional range. However, its application to felsic melts (> 68 wt% SiO2) is not recommended. Other advantages of this equation and differences when compared with previous models are discussed. More... »

PAGES

98

References to SciGraph publications

  • 2013-12. The effect of titanium and phosphorus on ferric/ferrous ratio in silicate melts: an experimental study in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 1991. Relations Between Structure, Redox Equilibria of Iron, and Properties of Magmatic Liquids in PHYSICAL CHEMISTRY OF MAGMAS
  • 2015-02. Effects of melt composition on Fe3+/Fe2+ in silicate melts: a step to model ferric/ferrous ratio in multicomponent systems in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 1995-06. The effect of dissolved water on the oxidation state of iron in natural silicate liquids in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 2017-05. Effects of strong network modifiers on Fe3+/Fe2+ in silicate melts: an experimental study in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 1993-03. The role of phosphorus in rhyolitic liquids as determined from the homogeneous iron redox equilibrium in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 2010-09. Ferric-ferrous ratio in liquid iron oxides: Analysis and applications to natural basaltic melts in PETROLOGY
  • 1991-07. The compressibility of silicate liquids containing Fe2O3 and the effect of composition, temperature, oxygen fugacity and pressure on their redox states in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 2007-11. Experimental study of the influence of SiO2 on the solubility of cobalt and iron in silicate melts in PETROLOGY
  • 1981-02. Ferric-ferrous equilibria in natural silicate liquids at 1 bar in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 1985-07. A comparison of iron redox ratios in silicate glasses determined by wet-chemical and 57Fe Mössbauer resonant absorption methods in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 1983-08. The ferric-ferrous ratio of natural silicate liquids equilibrated in air in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • 2004-07. Mössbauer spectroscopic determination of Fe3+/Fe2+ in synthetic basaltic glass: a test of empirical fO2 equations under superliquidus and subliquidus conditions in CONTRIBUTIONS TO MINERALOGY AND PETROLOGY
  • Identifiers

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    http://scigraph.springernature.com/pub.10.1007/s00410-018-1524-8

    DOI

    http://dx.doi.org/10.1007/s00410-018-1524-8

    DIMENSIONS

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