Transport properties of high albite crystals, near-endmember feldspar and pyroxene glasses, and their melts to high temperature View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2009-09

AUTHORS

Anne M. Hofmeister, Alan G. Whittington, Maik Pertermann

ABSTRACT

Thermal diffusivity (D) was measured using laser-flash analysis (LFA) from oriented single-crystal albite and glasses near LiAlSi3O8, NaAlSi3O8, CaAl2Si2O8, LiAlSi2O6 and CaMgSi2O6 compositions. Viscosity measurements of the supercooled liquids, over 2.6 × 108 to 8.9 × 1012 Pa s, confirm strongly non-Arrhenian behavior for CaAl2Si2O8, and CaMgSi2O6, and near-Arrhenian behavior for the others. As T increases, Dglass decreases, approaching a constant near 1,000 K. Upon crossing the glass transition, D decreases rapidly. For feldspars, D for the melt is ~15% below D of the bulk crystal, whereas for pyroxenes, this difference is ~40%. Thermal conductivity (klat = ρCPD) of crystals decreases with increasing T, but klat of glasses increases with T because heat capacity (CP) increases with T more strongly than density (ρ) and D decrease. For feldspars, klat for the melt is ~10% below that of the bulk crystal or glass, whereas this decrease for pyroxene is ~50%. Therefore, melting substantially impedes heat transport, providing positive thermal feedback that could promote further melting. More... »

PAGES

381

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00410-009-0388-3

DOI

http://dx.doi.org/10.1007/s00410-009-0388-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1032902625


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    "description": "Thermal diffusivity (D) was measured using laser-flash analysis (LFA) from oriented single-crystal albite and glasses near LiAlSi3O8, NaAlSi3O8, CaAl2Si2O8, LiAlSi2O6 and CaMgSi2O6 compositions. Viscosity measurements of the supercooled liquids, over 2.6 \u00d7 108 to 8.9 \u00d7 1012 Pa s, confirm strongly non-Arrhenian behavior for CaAl2Si2O8, and CaMgSi2O6, and near-Arrhenian behavior for the others. As T increases, Dglass decreases, approaching a constant near 1,000 K. Upon crossing the glass transition, D decreases rapidly. For feldspars, D for the melt is ~15% below D of the bulk crystal, whereas for pyroxenes, this difference is ~40%. Thermal conductivity (klat = \u03c1CPD) of crystals decreases with increasing T, but klat of glasses increases with T because heat capacity (CP) increases with T more strongly than density (\u03c1) and D decrease. For feldspars, klat for the melt is ~10% below that of the bulk crystal or glass, whereas this decrease for pyroxene is ~50%. Therefore, melting substantially impedes heat transport, providing positive thermal feedback that could promote further melting.", 
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