Transport properties of low-sanidine single-crystals, glasses and melts at high temperature View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2008-06

AUTHORS

Maik Pertermann, Alan G. Whittington, Anne M. Hofmeister, Frank J. Spera, John Zayak

ABSTRACT

Thermal diffusivity (D) was measured using laser-flash analysis from oriented single-crystal low-sanidine (K0.92Na0.08Al0.99Fe3+0.005Si2.95O8), and three glasses near KAlSi3O8. Viscosity measurements of the three supercooled liquids, in the range 106.8 to 1012.3 Pa s, confirm near-Arrhenian behavior, varying subtly with composition. For crystal and glass, D decreases with T, approaching a constant near 1,000 K: Dsat ∼ 0.65 ± 0.3 mm2 s−1 for bulk crystal and ∼0.53 ± 0.03 mm2 s−1 for the glass. A rapid decrease near 1,400 K is consistent with crossing the glass transition. Melt behavior is approximated by D = 0.475 ± 0.01 mm2 s−1. Thermal conductivity (klat) of glass, calculated using previous heat capacity (CP) and new density data, increases with T because CP strongly increases with T. For melt, klat reaches a plateau near 1.45 W m−1 K−1, and is always below klat of the crystal. Melting of potassium feldspars impedes heat transport, providing positive thermal feedback that may promote further melting in continental crust. More... »

PAGES

689-702

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URI

http://scigraph.springernature.com/pub.10.1007/s00410-007-0265-x

DOI

http://dx.doi.org/10.1007/s00410-007-0265-x

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41 schema:description Thermal diffusivity (D) was measured using laser-flash analysis from oriented single-crystal low-sanidine (K0.92Na0.08Al0.99Fe3+0.005Si2.95O8), and three glasses near KAlSi3O8. Viscosity measurements of the three supercooled liquids, in the range 106.8 to 1012.3 Pa s, confirm near-Arrhenian behavior, varying subtly with composition. For crystal and glass, D decreases with T, approaching a constant near 1,000 K: Dsat ∼ 0.65 ± 0.3 mm2 s−1 for bulk crystal and ∼0.53 ± 0.03 mm2 s−1 for the glass. A rapid decrease near 1,400 K is consistent with crossing the glass transition. Melt behavior is approximated by D = 0.475 ± 0.01 mm2 s−1. Thermal conductivity (klat) of glass, calculated using previous heat capacity (CP) and new density data, increases with T because CP strongly increases with T. For melt, klat reaches a plateau near 1.45 W m−1 K−1, and is always below klat of the crystal. Melting of potassium feldspars impedes heat transport, providing positive thermal feedback that may promote further melting in continental crust.
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