Electromagnetic interaction of fluorophores with designed two-dimensional silver nanoparticle arrays View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2001-09

AUTHORS

H. Ditlbacher, N. Felidj, J.R. Krenn, B. Lamprecht, A. Leitner, F.R. Aussenegg

ABSTRACT

. We study the fluorescence enhancement of dye molecules adsorbed on regular two-dimensional arrays of designed silver nanoparticles. The silver particles show two orthogonal optical resonances at different wavelengths because of their elongated shape. The short-wavelength resonance was designed to fit to the absorption maximum of the fluorophore. When the excitation light drives the short-wavelength resonance, the measured fluorescence intensity is strongly enhanced compared to that for the orthogonal particle orientation. This shows directly a strong electromagnetic coupling between the nanoparticles and the fluorophore. Additionally enhanced photochemical bleaching is observed due to the interaction of fluorophores with the particles. Using a rate model describing the fluorescence enhancement and the bleaching enhancement, an average value for the particle-induced increase in the radiative fluorescence rate is obtained, together with a lower limit for the averaged particle-induced field intensity enhancement factor. More... »

PAGES

373-377

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s003400100700

DOI

http://dx.doi.org/10.1007/s003400100700

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1005780086


Indexing Status Check whether this publication has been indexed by Scopus and Web Of Science using the SN Indexing Status Tool
Incoming Citations Browse incoming citations for this publication using opencitations.net

JSON-LD is the canonical representation for SciGraph data.

TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT

[
  {
    "@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json", 
    "about": [
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/02", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Physical Sciences", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/09", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Engineering", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0205", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Optical Physics", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0906", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Electrical and Electronic Engineering", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0913", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Mechanical Engineering", 
        "type": "DefinedTerm"
      }
    ], 
    "author": [
      {
        "affiliation": {
          "alternateName": "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT", 
          "id": "http://www.grid.ac/institutes/grid.5110.5", 
          "name": [
            "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Ditlbacher", 
        "givenName": "H.", 
        "id": "sg:person.0632253671.78", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0632253671.78"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Interfaces, Traitements, Organisation et Dynamique des Systemes, Universit\u00e9 Paris 7, CNRS UPRES.A, Paris, France, FR", 
          "id": "http://www.grid.ac/institutes/grid.508487.6", 
          "name": [
            "Interfaces, Traitements, Organisation et Dynamique des Systemes, Universit\u00e9 Paris 7, CNRS UPRES.A, Paris, France, FR"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Felidj", 
        "givenName": "N.", 
        "id": "sg:person.01265456317.19", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01265456317.19"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT", 
          "id": "http://www.grid.ac/institutes/grid.5110.5", 
          "name": [
            "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Krenn", 
        "givenName": "J.R.", 
        "id": "sg:person.01036636616.67", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01036636616.67"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT", 
          "id": "http://www.grid.ac/institutes/grid.5110.5", 
          "name": [
            "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Lamprecht", 
        "givenName": "B.", 
        "id": "sg:person.010525000635.09", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010525000635.09"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT", 
          "id": "http://www.grid.ac/institutes/grid.5110.5", 
          "name": [
            "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Leitner", 
        "givenName": "A.", 
        "id": "sg:person.01363552660.00", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01363552660.00"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT", 
          "id": "http://www.grid.ac/institutes/grid.5110.5", 
          "name": [
            "Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schr\u00f6dinger Institute for Nanoscale Research, Graz, Austria, AT"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Aussenegg", 
        "givenName": "F.R.", 
        "id": "sg:person.0106671207.22", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0106671207.22"
        ], 
        "type": "Person"
      }
    ], 
    "datePublished": "2001-09", 
    "datePublishedReg": "2001-09-01", 
    "description": "Abstract. We study the fluorescence enhancement of dye molecules adsorbed on regular two-dimensional arrays of designed silver nanoparticles. The silver particles show two orthogonal optical resonances at different wavelengths because of their elongated shape. The short-wavelength resonance was designed to fit to the absorption maximum of the fluorophore. When the excitation light drives the short-wavelength resonance, the measured fluorescence intensity is strongly enhanced compared to that for the orthogonal particle orientation. This shows directly a strong electromagnetic coupling between the nanoparticles and the fluorophore. Additionally enhanced photochemical bleaching is observed due to the interaction of fluorophores with the particles. Using a rate model describing the fluorescence enhancement and the bleaching enhancement, an average value for the particle-induced increase in the radiative fluorescence rate is obtained, together with a lower limit for the averaged particle-induced field intensity enhancement factor.", 
    "genre": "article", 
    "id": "sg:pub.10.1007/s003400100700", 
    "isAccessibleForFree": false, 
    "isPartOf": [
      {
        "id": "sg:journal.1312262", 
        "issn": [
          "0946-2171", 
          "1432-0649"
        ], 
        "name": "Applied Physics B", 
        "publisher": "Springer Nature", 
        "type": "Periodical"
      }, 
      {
        "issueNumber": "4", 
        "type": "PublicationIssue"
      }, 
      {
        "type": "PublicationVolume", 
        "volumeNumber": "73"
      }
    ], 
    "keywords": [
      "short-wavelength resonance", 
      "fluorescence enhancement", 
      "two-dimensional silver nanoparticle arrays", 
      "interactions of fluorophores", 
      "silver nanoparticle arrays", 
      "dye molecules", 
      "silver nanoparticles", 
      "silver particles", 
      "nanoparticle arrays", 
      "absorption maximum", 
      "fluorophores", 
      "photochemical bleaching", 
      "fluorescence intensity", 
      "enhancement factor", 
      "nanoparticles", 
      "fluorescence rate", 
      "lower limit", 
      "excitation light", 
      "strong electromagnetic coupling", 
      "two-dimensional array", 
      "intensity enhancement factor", 
      "field intensity enhancement factor", 
      "resonance", 
      "particles", 
      "molecules", 
      "particle-induced increase", 
      "optical resonances", 
      "enhancement", 
      "interaction", 
      "different wavelengths", 
      "particle orientation", 
      "bleaching", 
      "limit", 
      "coupling", 
      "rate model", 
      "array", 
      "wavelength", 
      "light", 
      "orientation", 
      "intensity", 
      "maximum", 
      "shape", 
      "average value", 
      "values", 
      "increase", 
      "rate", 
      "electromagnetic coupling", 
      "electromagnetic interactions", 
      "model", 
      "factors"
    ], 
    "name": "Electromagnetic interaction of fluorophores with designed two-dimensional silver nanoparticle arrays", 
    "pagination": "373-377", 
    "productId": [
      {
        "name": "dimensions_id", 
        "type": "PropertyValue", 
        "value": [
          "pub.1005780086"
        ]
      }, 
      {
        "name": "doi", 
        "type": "PropertyValue", 
        "value": [
          "10.1007/s003400100700"
        ]
      }
    ], 
    "sameAs": [
      "https://doi.org/10.1007/s003400100700", 
      "https://app.dimensions.ai/details/publication/pub.1005780086"
    ], 
    "sdDataset": "articles", 
    "sdDatePublished": "2022-09-02T15:48", 
    "sdLicense": "https://scigraph.springernature.com/explorer/license/", 
    "sdPublisher": {
      "name": "Springer Nature - SN SciGraph project", 
      "type": "Organization"
    }, 
    "sdSource": "s3://com-springernature-scigraph/baseset/20220902/entities/gbq_results/article/article_316.jsonl", 
    "type": "ScholarlyArticle", 
    "url": "https://doi.org/10.1007/s003400100700"
  }
]
 

Download the RDF metadata as:  json-ld nt turtle xml License info

HOW TO GET THIS DATA PROGRAMMATICALLY:

JSON-LD is a popular format for linked data which is fully compatible with JSON.

curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1007/s003400100700'

N-Triples is a line-based linked data format ideal for batch operations.

curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1007/s003400100700'

Turtle is a human-readable linked data format.

curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1007/s003400100700'

RDF/XML is a standard XML format for linked data.

curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1007/s003400100700'


 

This table displays all metadata directly associated to this object as RDF triples.

157 TRIPLES      20 PREDICATES      78 URIs      67 LITERALS      6 BLANK NODES

Subject Predicate Object
1 sg:pub.10.1007/s003400100700 schema:about anzsrc-for:02
2 anzsrc-for:0205
3 anzsrc-for:09
4 anzsrc-for:0906
5 anzsrc-for:0913
6 schema:author Nb775a93a2439473c8e57520bbc6fd83b
7 schema:datePublished 2001-09
8 schema:datePublishedReg 2001-09-01
9 schema:description Abstract. We study the fluorescence enhancement of dye molecules adsorbed on regular two-dimensional arrays of designed silver nanoparticles. The silver particles show two orthogonal optical resonances at different wavelengths because of their elongated shape. The short-wavelength resonance was designed to fit to the absorption maximum of the fluorophore. When the excitation light drives the short-wavelength resonance, the measured fluorescence intensity is strongly enhanced compared to that for the orthogonal particle orientation. This shows directly a strong electromagnetic coupling between the nanoparticles and the fluorophore. Additionally enhanced photochemical bleaching is observed due to the interaction of fluorophores with the particles. Using a rate model describing the fluorescence enhancement and the bleaching enhancement, an average value for the particle-induced increase in the radiative fluorescence rate is obtained, together with a lower limit for the averaged particle-induced field intensity enhancement factor.
10 schema:genre article
11 schema:isAccessibleForFree false
12 schema:isPartOf N12c710dc21554e61a8d20bfd4bfdf9ef
13 Nca5612d7e491444da371ecdd0d50603a
14 sg:journal.1312262
15 schema:keywords absorption maximum
16 array
17 average value
18 bleaching
19 coupling
20 different wavelengths
21 dye molecules
22 electromagnetic coupling
23 electromagnetic interactions
24 enhancement
25 enhancement factor
26 excitation light
27 factors
28 field intensity enhancement factor
29 fluorescence enhancement
30 fluorescence intensity
31 fluorescence rate
32 fluorophores
33 increase
34 intensity
35 intensity enhancement factor
36 interaction
37 interactions of fluorophores
38 light
39 limit
40 lower limit
41 maximum
42 model
43 molecules
44 nanoparticle arrays
45 nanoparticles
46 optical resonances
47 orientation
48 particle orientation
49 particle-induced increase
50 particles
51 photochemical bleaching
52 rate
53 rate model
54 resonance
55 shape
56 short-wavelength resonance
57 silver nanoparticle arrays
58 silver nanoparticles
59 silver particles
60 strong electromagnetic coupling
61 two-dimensional array
62 two-dimensional silver nanoparticle arrays
63 values
64 wavelength
65 schema:name Electromagnetic interaction of fluorophores with designed two-dimensional silver nanoparticle arrays
66 schema:pagination 373-377
67 schema:productId N9bbea95753e74eceb9adf24a47d20dbd
68 Nde6b4d434c7c421fa431bb195ca6cf07
69 schema:sameAs https://app.dimensions.ai/details/publication/pub.1005780086
70 https://doi.org/10.1007/s003400100700
71 schema:sdDatePublished 2022-09-02T15:48
72 schema:sdLicense https://scigraph.springernature.com/explorer/license/
73 schema:sdPublisher N14cdf27b95c84087aa05594ec759a198
74 schema:url https://doi.org/10.1007/s003400100700
75 sgo:license sg:explorer/license/
76 sgo:sdDataset articles
77 rdf:type schema:ScholarlyArticle
78 N12c710dc21554e61a8d20bfd4bfdf9ef schema:issueNumber 4
79 rdf:type schema:PublicationIssue
80 N14cdf27b95c84087aa05594ec759a198 schema:name Springer Nature - SN SciGraph project
81 rdf:type schema:Organization
82 N1e51dedb14de4e15be13d42b450f14d9 rdf:first sg:person.01363552660.00
83 rdf:rest N995a21a381df45989b36d03e0dc46a1c
84 N35160c732ec24997b1654b25394341f0 rdf:first sg:person.01036636616.67
85 rdf:rest N55659c750fde4a3d80ef38ac5038e9f8
86 N55659c750fde4a3d80ef38ac5038e9f8 rdf:first sg:person.010525000635.09
87 rdf:rest N1e51dedb14de4e15be13d42b450f14d9
88 N995a21a381df45989b36d03e0dc46a1c rdf:first sg:person.0106671207.22
89 rdf:rest rdf:nil
90 N9bbea95753e74eceb9adf24a47d20dbd schema:name doi
91 schema:value 10.1007/s003400100700
92 rdf:type schema:PropertyValue
93 Nab613a09b91e4aacb49f28c31aa8f717 rdf:first sg:person.01265456317.19
94 rdf:rest N35160c732ec24997b1654b25394341f0
95 Nb775a93a2439473c8e57520bbc6fd83b rdf:first sg:person.0632253671.78
96 rdf:rest Nab613a09b91e4aacb49f28c31aa8f717
97 Nca5612d7e491444da371ecdd0d50603a schema:volumeNumber 73
98 rdf:type schema:PublicationVolume
99 Nde6b4d434c7c421fa431bb195ca6cf07 schema:name dimensions_id
100 schema:value pub.1005780086
101 rdf:type schema:PropertyValue
102 anzsrc-for:02 schema:inDefinedTermSet anzsrc-for:
103 schema:name Physical Sciences
104 rdf:type schema:DefinedTerm
105 anzsrc-for:0205 schema:inDefinedTermSet anzsrc-for:
106 schema:name Optical Physics
107 rdf:type schema:DefinedTerm
108 anzsrc-for:09 schema:inDefinedTermSet anzsrc-for:
109 schema:name Engineering
110 rdf:type schema:DefinedTerm
111 anzsrc-for:0906 schema:inDefinedTermSet anzsrc-for:
112 schema:name Electrical and Electronic Engineering
113 rdf:type schema:DefinedTerm
114 anzsrc-for:0913 schema:inDefinedTermSet anzsrc-for:
115 schema:name Mechanical Engineering
116 rdf:type schema:DefinedTerm
117 sg:journal.1312262 schema:issn 0946-2171
118 1432-0649
119 schema:name Applied Physics B
120 schema:publisher Springer Nature
121 rdf:type schema:Periodical
122 sg:person.01036636616.67 schema:affiliation grid-institutes:grid.5110.5
123 schema:familyName Krenn
124 schema:givenName J.R.
125 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01036636616.67
126 rdf:type schema:Person
127 sg:person.010525000635.09 schema:affiliation grid-institutes:grid.5110.5
128 schema:familyName Lamprecht
129 schema:givenName B.
130 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010525000635.09
131 rdf:type schema:Person
132 sg:person.0106671207.22 schema:affiliation grid-institutes:grid.5110.5
133 schema:familyName Aussenegg
134 schema:givenName F.R.
135 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0106671207.22
136 rdf:type schema:Person
137 sg:person.01265456317.19 schema:affiliation grid-institutes:grid.508487.6
138 schema:familyName Felidj
139 schema:givenName N.
140 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01265456317.19
141 rdf:type schema:Person
142 sg:person.01363552660.00 schema:affiliation grid-institutes:grid.5110.5
143 schema:familyName Leitner
144 schema:givenName A.
145 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01363552660.00
146 rdf:type schema:Person
147 sg:person.0632253671.78 schema:affiliation grid-institutes:grid.5110.5
148 schema:familyName Ditlbacher
149 schema:givenName H.
150 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0632253671.78
151 rdf:type schema:Person
152 grid-institutes:grid.508487.6 schema:alternateName Interfaces, Traitements, Organisation et Dynamique des Systemes, Université Paris 7, CNRS UPRES.A, Paris, France, FR
153 schema:name Interfaces, Traitements, Organisation et Dynamique des Systemes, Université Paris 7, CNRS UPRES.A, Paris, France, FR
154 rdf:type schema:Organization
155 grid-institutes:grid.5110.5 schema:alternateName Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schrödinger Institute for Nanoscale Research, Graz, Austria, AT
156 schema:name Institute for Experimental Physics, Karl-Franzens-University Graz, and Erwin-Schrödinger Institute for Nanoscale Research, Graz, Austria, AT
157 rdf:type schema:Organization
 




Preview window. Press ESC to close (or click here)


...