Characterization of ultrafast plasmon dynamics in individual gold bowtie by time-resolved photoemission electron microscopy View Full Text


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Article Info

DATE

2018-12-03

AUTHORS

Yulu Qin, Boyu Ji, Xiaowei Song, Jingquan Lin

ABSTRACT

We report on the investigation of ultrafast dynamics of the plasmonic field in individual gold bowtie nanostructure by combining interferometric time-resolved photoemission electron microscopy with a damped harmonic oscillator model. We experimentally obtain different plasmon dephasing times in the tips of the bowtie nanostructure. In the meantime, we demonstrate that the experimental time-resolved photoemission signal can be used to directly compare resonance frequency and dephasing time of different hot spots. In addition, we find that the plasmon field, which is extracted from the photoemission signal, initially oscillates at the laser field frequency, and finally develops into its eigenfrequency after experiencing a few periods of frequency fluctuation due to the competition between forced and autonomous oscillation of the plasmons. More... »

PAGES

3

References to SciGraph publications

  • 2007-06-09. Phase propagation of localized surface plasmons probed by time-resolved photoemission electron microscopy in APPLIED PHYSICS A
  • 2013-12-20. Direct imaging of the near field and dynamics of surface plasmon resonance on gold nanostructures using photoemission electron microscopy in LIGHT: SCIENCE & APPLICATIONS
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  • 1999-03. SHG studies of plasmon dephasing in nanoparticles in APPLIED PHYSICS B
  • 1997-02. Femtosecond decay-time measurement of electron-plasma oscillation in nanolithographically designed silver particles in APPLIED PHYSICS B
  • 2010-06-01. Damping of the localized surface plasmon polariton resonance of gold nanoparticles in APPLIED PHYSICS B
  • 2011-10-16. Plasmonic generation of ultrashort extreme-ultraviolet light pulses in NATURE PHOTONICS
  • 2014-01-30. Plasmon-induced hot-electron generation at nanoparticle/metal-oxide interfaces for photovoltaic and photocatalytic devices in NATURE PHOTONICS
  • 2016-06-30. Determination of local optical response functions of nanostructures with increasing complexity by using single and coupled Lorentzian oscillator models in APPLIED PHYSICS B
  • 2016-09-09. Electron microscopy methods for space-, energy-, and time-resolved plasmonics in FRONTIERS OF PHYSICS
  • 2017-11-03. Cavity-assisted ultrafast long-range periodic energy transfer between plasmonic nanoantennas in LIGHT: SCIENCE & APPLICATIONS
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    http://scigraph.springernature.com/pub.10.1007/s00340-018-7112-9

    DOI

    http://dx.doi.org/10.1007/s00340-018-7112-9

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