Rapid, broadband spectroscopic temperature measurement of CO2 using VIPA spectroscopy View Full Text


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Article Info

DATE

2016-04

AUTHORS

Andrew Klose, Gabriel Ycas, Flavio C. Cruz, Daniel L. Maser, Scott A. Diddams

ABSTRACT

Time-resolved spectroscopic temperature measurements of a sealed carbon dioxide sample cell were realized with an optical frequency comb combined with a two-dimensional dispersive spectrometer. A supercontinuum laser source based on an erbium fiber mode-locked laser was employed to generate coherent light around 2000 nm (5000cm-1). The laser was passed through a 12-cm-long cell containing CO2, and the transmitted light was analyzed in a virtually imaged phased array-based spectrometer. Broadband spectra spanning more than 100cm-1 with a spectral resolution of roughly 0.075cm-1 (2.2 GHz) were acquired with an integration period of 2 ms. The temperature of the CO2 sample was deduced from fitting a modeled spectrum to the line intensities of the experimentally acquired spectrum. Temperature dynamics on the timescale of milliseconds were observed with a temperature resolution of 2.6 K. The spectroscopically deduced temperatures agreed with temperatures of the sample cell measured with a thermistor. Potential applications of this technique include quantitative measurement of carbon dioxide concentration and temperature dynamics in gas-phase chemical reactions (e.g., combustion) and plasma diagnostics. More... »

PAGES

78

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00340-016-6349-4

DOI

http://dx.doi.org/10.1007/s00340-016-6349-4

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https://app.dimensions.ai/details/publication/pub.1009544660


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