Bundling influence on ultrafast optical nonlinearities of single-walled carbon nanotubes in suspension and composite film View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2009-09

AUTHORS

H. W. Lee, J. H. Yim, A. J. Kiran, I. H. Baek, S. Lee, D.-I. Yeom, Y. H. Ahn, K. Kim, J. Lee, H. Lim, F. Rotermund

ABSTRACT

Nonlinear optical characteristics of single-walled carbon nanotubes (SWCNTs) dispersed in dichlorobenzene and imbedded in polymer were investigated at 800 nm using the time-resolved optical Kerr gate technique. For systematic study of the influence of SWCNT bundling on optical nonlinearities, SWCNT solutions with different concentrations and a series of SWCNT/polymer composites deposited on glass substrates with different concentrations and thicknesses were prepared. The nonlinear response was comparable to the pulse duration of the laser used (∼90 fs) both in SWCNT solutions and SWCNT/polymer composites. Over three orders of magnitude enhancement was observed in the third-order nonlinear susceptibility of SWCNT/polymer composite film compared with that of SWCNT solution. An appreciable reduction of microscopic and macroscopic nonlinearities was observed with increasing SWCNT concentrations due to stronger bundling of SWCNTs. More... »

PAGES

157-162

References to SciGraph publications

Journal

TITLE

Applied Physics B

ISSUE

1

VOLUME

97

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00340-009-3532-x

DOI

http://dx.doi.org/10.1007/s00340-009-3532-x

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1006558458


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