Structure, dielectric behaviours, enhanced polarization responses and energy storage properties in (1 − x)SrTiO3–xBi(Mg1/2Ti1/2)O3 ceramics View Full Text


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Article Info

DATE

2018-12

AUTHORS

Yongxing Wei, Gang Xu, Changqing Jin, Yiming Zeng, Kang Yan, Siyuan Dong, Peng Li

ABSTRACT

In this work, ceramics of (1 − x)SrTiO3–xBi(Mg1/2Ti1/2)O3 (ST–BMT, x = 0.05–0.5) were successfully prepared. A single-phase perovskite structure is formed for all the compositions. The average structure is cubic at room temperature. The Raman analysis suggests that the 5 mol% BMT addition might cause the existence of the local tetragonal distortions at room temperature. All the compositions display a frequency-dependent and highly diffused dielectric anomaly. The BMT addition can effectively shift the freezing temperature (Tf), from ~ 32 K for x = 0.1 up to ~ 240 K for x = 0.5. The compositions with x = 0.4 and 0.5 show a small change in the relative permittivity (Δε′/ε373K′ < ± 15% at 1 kHz) and keep low values of the dielectric loss (tanδ < 0.01 for x = 0.01 at 1 kHz) in the temperature range of 373–523 K. The BMT addition induces an enhancement of the polarization maxima. Among the compositions, 0.7ST–0.3BMT shows the optimum energy storage performance (Wrec, 0.78 J/cm3). More... »

PAGES

862

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00339-018-2295-9

DOI

http://dx.doi.org/10.1007/s00339-018-2295-9

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41 schema:description In this work, ceramics of (1 − x)SrTiO3–xBi(Mg1/2Ti1/2)O3 (ST–BMT, x = 0.05–0.5) were successfully prepared. A single-phase perovskite structure is formed for all the compositions. The average structure is cubic at room temperature. The Raman analysis suggests that the 5 mol% BMT addition might cause the existence of the local tetragonal distortions at room temperature. All the compositions display a frequency-dependent and highly diffused dielectric anomaly. The BMT addition can effectively shift the freezing temperature (Tf), from ~ 32 K for x = 0.1 up to ~ 240 K for x = 0.5. The compositions with x = 0.4 and 0.5 show a small change in the relative permittivity (Δε′/ε373K′ < ± 15% at 1 kHz) and keep low values of the dielectric loss (tanδ < 0.01 for x = 0.01 at 1 kHz) in the temperature range of 373–523 K. The BMT addition induces an enhancement of the polarization maxima. Among the compositions, 0.7ST–0.3BMT shows the optimum energy storage performance (Wrec, 0.78 J/cm3).
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