Electrical properties, structure, and surface morphology of poly(p-xylylene)–silver nanocomposites synthesized by low-temperature vapor deposition polymerization View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2013-02

AUTHORS

Dmitry R. Streltsov, Karen A. Mailyan, Alexey V. Gusev, Ilya A. Ryzhikov, Natalia A. Erina, Chanmin Su, Andrey V. Pebalk, Sergei A. Ozerin, Sergei N. Chvalun

ABSTRACT

The crystalline structure, surface morphology, electrical, and optical properties of thin films of nanocomposites consisting of silver nanoparticles embedded in poly(p-xylylene) matrix prepared by low-temperature vapor deposition polymerization were studied. Depending on the filler content, the average size of silver nanoparticles varied from 2 to 5 nm for nanocomposites with 2 and 12 vol.% of silver, correspondingly. The optical adsorption in the visible region due to surface plasmon resonance also exhibited a clear correlation from silver content, revealing a red shift of the adsorption peak with the increase of the metal concentration. The temperature dependences of the dc resistance of pure p-xylylene condensate and p-xylylene–silver cocondensates during polymerization as well as temperature dependences of the formed poly(p-xylylene)–silver nanocomposites were examined. The observed variation of the temperature dependences of electrical resistance as a function of silver concentration are attributed to different conduction mechanisms and correlated with the structure of the composites. The wide-angle X-ray scattering and AFM measurements consistently show a strong effect of silver content on the nanocomposite structure. The evolution of the size of silver nanoparticles by thermal annealing was demonstrated. More... »

PAGES

413-422

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00339-012-7220-z

DOI

http://dx.doi.org/10.1007/s00339-012-7220-z

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1053460775


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