Electronic state of nanodiamond/graphite interfaces View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2005-07

AUTHORS

A.V. Okotrub, L.G. Bulusheva, V.L. Kuznetsov, A.V. Gusel’nikov, A.L. Chuvilin

ABSTRACT

The electronic state of nanodiamond/graphite interfaces in samples prepared by annealing of nanodiamonds (ND) at 1150–1600 K has been probed using X-ray fluorescence spectroscopy and field-emission measurements. Comparison between [C]Kα spectra of ND before and after annealing revealed an enhancement of density of high-energy occupied states in the products. A quantum-chemical calculation using a carbon model showed that the observed states could originate from the electrons of dangling bonds produced by peeling of a graphitic shell from the (111) surface of a diamond particle. The developed graphitic layers screen the weakly bonding electrons, which results in a lowering of the efficiency of field-electron emission from the samples with an increase of annealing temperature. More... »

PAGES

393-398

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00339-004-2565-6

DOI

http://dx.doi.org/10.1007/s00339-004-2565-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1017503143


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