Impact of Land Use on the Mobility of Hg Species in Different Compartments of a Tropical Watershed in Brazil View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2017-09-09

AUTHORS

Clara Ayume Ito de Lima, Marcelo Gomes de Almeida, Inacio Abreu Pestana, Wanderley R. Bastos, Maria Cristina Nery do Nascimento Recktenvald, Cristina Maria Magalhães de Souza, Paulo Pedrosa

ABSTRACT

This study evaluated the levels of total Hg and CH3Hg+ from a comprehensive perspective, considering the retention, leaching, and deposition of these contaminants in the main compartments (soil, plant litter, and sediment) of three landscapes (Atlantic Forest, pasture, and agricultural area) in a watershed in northern Rio de Janeiro State, Brazil. Variables analyzed were total Hg, CH3Hg+, organic carbon, total nitrogen, grain size, and surface area. In soil samples, total Hg levels were the highest in agricultural soil followed by forest soil and pasture (97.3, 87.6, and 77.1 ng g−1, respectively), and CH3Hg+ was lower than 1.7%. Total Hg levels in leaf litter varied between 22.6 and 34.2 ng g−1, and CH3Hg+ was 4.37%. In sediment, Hg (60–180 ng g−1) and CH3Hg+ (<1%) indicate the transport of these contaminants from soils to this compartment and may be associated with soil use and cover. Multiple regressions were used to understand the dispersion of Hg species, and the effect of each variable varied with the landscape, showing that plant cover should not be ignored in investigations related to Hg species retention in a watershed. The landscapes surveyed in the present study clearly influence the quantitative and qualitative distribution of Hg species. On the other hand, anthropic processes associated with changes in soil use did not have any critical effects on the absolute levels of total Hg and CH3Hg+, meaning that the landscapes evaluated seem to represent the background concentration of these chemical species for the evaluated watershed. More... »

PAGES

578-592

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00244-017-0449-y

DOI

http://dx.doi.org/10.1007/s00244-017-0449-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1091511962

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/28889279


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