Characterization of nuclear fuels by ICP mass-spectrometric techniques View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2008-01

AUTHORS

Ines Günther-Leopold, Niko Kivel, Judith Kobler Waldis, Beat Wernli

ABSTRACT

Isotopic analyses of radioactive materials such as irradiated nuclear fuel are of major importance for the optimization of the nuclear fuel cycle and for safeguard aspects. Among the mass-spectrometric techniques available, inductively coupled plasma mass spectrometry (ICP-MS) and thermal ionization mass spectrometry are the most frequently applied methods for nuclear applications. Because of the low detection limits, the ability to analyze the isotopic composition of the elements and the applicability of the techniques for measuring stable as well as radioactive nuclides with similar sensitivity, both mass-spectrometric techniques are an excellent amendment to classical radioactivity counting methods. The paper describes selected applications of multicollector ICP-MS in combination with chromatographic separation techniques and laser ablation for the isotopic analysis of irradiated nuclear fuels. The advantages and limitations of the selected analytical technique for the characterization of such a heterogeneous sample matrix are discussed. More... »

PAGES

503-510

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s00216-007-1644-x

DOI

http://dx.doi.org/10.1007/s00216-007-1644-x

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1028001233

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/17924097


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