Influence of CF3H and CCl4 additives on acetylene detonation View Full Text


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Article Info

DATE

2014-03

AUTHORS

A. Drakon, A. Emelianov, A. Eremin

ABSTRACT

The influence of CF3H and CCl4 admixtures (known as detonation suppressors for combustible mixtures) on the development of acetylene detonation was experimentally investigated in a shock tube. The time-resolved images of detonation wave development and propagation were registered using a high-speed streak camera. Shock wave velocity and pressure profiles were measured by five calibrated piezoelectric gauges and the formation of condensed particles was detected by laser light extinction. The induction time of detonation development was determined as the moment of a pressure rise at the end plate of the shock tube. It was shown that CF3H additive had no influence on the induction time. For CCl4, a significant promoting effect was observed. A simplified kinetic model was suggested and characteristic rates of diacetylene C4H2 formation were estimated as the limiting stage of acetylene polymerisation. An analysis of the obtained data indicated that the promoting species is atomic chlorine formed by CCl4 pyrolysis, which interacts with acetylene and produces C2H radical, initiating a chain mechanism of acetylene decomposition. The results of kinetic modelling agree well with the experimental data. More... »

PAGES

231-237

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URI

http://scigraph.springernature.com/pub.10.1007/s00193-013-0453-8

DOI

http://dx.doi.org/10.1007/s00193-013-0453-8

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