Stretching necklaces View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2000-07

AUTHORS

T.A. Vilgis, A. Johner, J.F. Joanny

ABSTRACT

Polyelectrolytes in poor solvents show a necklace structure where collapsed polymer pearls are linked to stretched strings. In the present paper the elasticity of such chains is studied in detail. Different deformation regimes are addressed. The first is the continuous regime, where many pearls are present. A continuous force extension relationship is calculated. The main contribution comes from the tension balance and the electrostatic repulsion of consecutive pearls. The main correction term stems from the finite size of the pearls, which monitors their surface energy. For a finite amount of pearls discontinuous stretching is predicted. Finally counterion effects are discussed qualitatively. More... »

PAGES

289-300

Journal

TITLE

The European Physical Journal E

ISSUE

3

VOLUME

2

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/pl00013674

DOI

http://dx.doi.org/10.1007/pl00013674

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1046719324


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