Hyperfine interactions at 181Hf(→181Ta) impurities implanted in Er2O3 and Gd2O3: structural and electronic dependence of the EFG in bixbyite sesquioxides View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2001-07

AUTHORS

L.A. Errico, M. Rentería, A.F. Pasquevich, A.G. Bibiloni, K. Freitag

ABSTRACT

The time-differential-perturbed γ-γ angular-correlation technique (TDPAC) with ion-implanted 181Hf tracers has been applied to study the hyperfine interactions of 181Ta impurities in the cubic bixbyite structure of Er 2 O 3 and Gd 2 O 3 . The TDPAC experiments were performed in air in the temperature range 300-1073 K (in the case of Er 2 O 3 ) and 300-1173 K (in the case of Gd 2 O 3 ). Three electrical-quadrupole interactions were found in each oxide in the whole studied temperature range. Two of them were attributed to the electric-field gradients (EFG) acting on 181Ta probes substitutionally located on the two nonequivalent free-of-defects cation sites of the bixbyite structure. The EFG results are compared with predictions of the point-charge model and discussed together with previous results obtained with the probes 111Cd and 181Ta in other isomorphous sesquioxides. The temperature dependence of the hyperfine parameters for both oxides is also discussed in terms of dilatometric expansion data. More... »

PAGES

149-156

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/pl00011141

DOI

http://dx.doi.org/10.1007/pl00011141

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1029743747


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