Bioelectronics and biometallocatalysis for production of fuels and chemicals by photosynthetic water splitting View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

1995-09

AUTHORS

James Weifu Lee, Elias Greenbaum

ABSTRACT

By inserting metallocatalysts (such as platinum, osmium, or ruthenium) at the reducing site of photosystem I (PSI), electrons that emerge from PSI can be channeled to various redox reactions that could potentially produce fuels and chemicals (such as H2 and CH4, and so forth) instead of NADP+ reduction, as in natural photosynthesis. We have recently developed a technique to photoprecipitate metallocatalystsin situ at the reducing site of PSI in thylakoid membranes, using water-soluble hexachloroplatinate, hexachloroosmiate, and hexachlororuthenate at biological temperature and neutral pH. This technique combined with “rewiring” of photosynthesis is a potentially important new field of biometallocatalysis. Potential applications of biometallocatalysis will be addressed in this article. More... »

PAGES

295-305

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/bf02933433

DOI

http://dx.doi.org/10.1007/bf02933433

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1030563824


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