Magnetic properties of Nd3+ in Nd−Ba−Cu−O-compounds View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

1994-09

AUTHORS

P. Allenspach, J. Mesot, U. Staub, M. Guillaume, A. Furrer, S. -I. Yoo, M. J. Kramer, R. W. McCallum, H. Maletta, H. Blank, H. Mutka, R. Osborn, M. Arai, Z. Bowden, A. D. Taylor

ABSTRACT

Neutron diffraction, neutron spectroscopy and magnetization measurements have been employed to study the structural, electronic, and magnetic behavior of eleven compounds with the general formula Nd1+yCavBa2−y−vCu3Ox (0≦y≦0.5; 0≦v≦0.25; 6≦x≦7). The structure turned out to react to oxygen reduction similar as other 123-compounds, yielding discontinuities close to the metal-insulator-transition and the well-known relations of bond lengths as a function ofTc. The crystalline electric field (CEF) interaction, splitting the 10-fold degenerate ground-state J-multiplet of the Nd3+-ions into five doublet states, was investigated by neutron spectroscopy. The derived CEF parameters have been used to determine changes in the electronic surroundings of the Nd3+ ions. In addition, with the help of the CEF parameters the thermodynamic magnetic properties of these compounds were calculated which turn out to be in good agreement with the experimental data. More... »

PAGES

301-310

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/bf01343957

DOI

http://dx.doi.org/10.1007/bf01343957

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1035691484


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