Oxidation of methanol at copper surfaces View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

1996-03

AUTHORS

A. F. Carley, A. W. Owens, M. K. Rajumon, M. W. Roberts, S. D. Jackson

ABSTRACT

The role of preadsorbed oxygen present at Cu(111), Cu(110) and polycrystalline surfaces in the oxidation of methanol has been investigated by X-ray and electron energy loss spectroscopies. In addition to the well established formation of methoxy species and its subsequent decomposition and desorption as formaldehyde, a second reaction pathway to surface formate is present. The latter is temperature dependent being undetectable at 260 K at a polycrystalline surface but occurs at a significant rate at 295 K and above. The limitations of experimental data for methanol oxidation by temperature programmed desorption and molecular beam techniques are discussed. More... »

PAGES

79-87

Journal

TITLE

Catalysis Letters

ISSUE

1-2

VOLUME

37

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/bf00813523

DOI

http://dx.doi.org/10.1007/bf00813523

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1013420568


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