Delocalization model of regioselectivity and reactivity of free radicals in reactions of addition to olefins View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

1987-03

AUTHORS

S. V. Volovik, G. G. Dyadyusha, V. I. Staninets

ABSTRACT

On the basis of the concept of polarity (“philicity”) of free radicals as proposed by the authors, within the framework of methods of qualitative surfaces of potential energy (linear combinations of configurations of fragments) and stabilization energy, an effective model has been developed for the regioselectivity and reactivity of radicals in processes of addition. A critical examination is made of certain key aspects of the change in regiochemistry and reactivity with changes in the electronic structure of the free radical and substrate. The dominant trends in regioselectivity and reactivity in processes of free-radical addition to olefins are controlled by electronic effects and can be predicted by analyzing interactions of diabatic potential energy surfaces or orbital interactions for a system consisting of a free radical and an unsaturated substrate. More... »

PAGES

128-140

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/bf00534572

DOI

http://dx.doi.org/10.1007/bf00534572

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1015396688


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