Rotaxanes and Catenanes in Action View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

1996

AUTHORS

J.-C. Chambron , C. O. Dietrich-Buchecker , A. Harriman , V. Heitz , A. Livoreil , J.-P. Sauvage

ABSTRACT

Not only are rotaxanes and catenanes aesthetically and topologically attractive molecules, but they can also be used as functional systems, able to undergo electronic and molecular motions under the action of an external stimulus. Porphyrin-stoppered rotaxanes are functional models of the photosynthetic Reaction Centre, leading to ultrafast interporphyrin electron transfer under light irradiation. Interestingly, the efficiency of the process strongly relies on the rotaxane nature of the compound, being mostly determined by the properties of the central transition metal complex. Different is the function of a non-symmetrical copper catenate, consisting of a two-coordination site ring interlocked to a one-chelate incorporating cycle. The oxidation state of the copper centre (I or II) entirely determines the set of ligands coordinated to the metal. Oxidizing or reducing the central copper atom thus induces a complete gliding motion of one cycle within the other. This process can be regarded as electrochemically triggerred swinging of the copper catenate. More... »

PAGES

1-8

References to SciGraph publications

Book

TITLE

Magnetism: A Supramolecular Function

ISBN

978-90-481-4730-4
978-94-015-8707-5

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-94-015-8707-5_1

DOI

http://dx.doi.org/10.1007/978-94-015-8707-5_1

DIMENSIONS

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