Theoretical Design of Organic Chromophores with Large Two-Photon Absorption Cross-Sections View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2000

AUTHORS

Marius Albota , David Beljonne , Jean-Luc Brédas , Jeffrey E. Ehrlich , Jia-Ying Fu , Ahmed A. Heikal , Samuel Hess , Thierry Kogej , Michael D. Levin , Seth R. Marder , Dianne McCordMaughon , Joseph W. Perry , Harald Röckel , Mariacristina Rumi , Girija Subramaniam , Watt W. Webb , Xiang-Li Wu , Chris Xu

ABSTRACT

Design strategies and structure-property relationships for two-photon absorption in conjugated molecules are described on the basis of correlated quantum-chemical calculations. We first focus on stilbene derivatives with centrosymmetric structures. We found that derivatization of the conjugated molecule with electroactive groups in a quadrupolarlike arrangement leads to a large increase in the two-photon absorption cross section, δ. Quantum-chemical description provides rich insight into the mechanisms for the two-photon absorption phenomenon. More... »

PAGES

53-65

Book

TITLE

Multiphoton and Light Driven Multielectron Processes in Organics: New Phenomena, Materials and Applications

ISBN

978-0-7923-6272-2
978-94-011-4056-0

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-94-011-4056-0_5

DOI

http://dx.doi.org/10.1007/978-94-011-4056-0_5

DIMENSIONS

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