High Pressure and Superconductivity: Intercalated Graphite Cac6 as a Model System View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2010-05-24

AUTHORS

A. Gauzzi , N. Bendiab , M. D’Astuto , B. Canny , M. Calandra , F. Mauri , G. Loupias , S. Takashima , H. Takagi , N. Takeshita , C. Terakura , N. Emery , C. Herold , PH. Lagrange , M. Hanfland , M. Mezouar

ABSTRACT

Superconducting CaC6 is found to exhibit two important pressure effects: (i) a large P-induced Tc enhancement up to 15.1 K at 7.5 GPa, the highest Tc value hitherto reported for graphite intercalated compounds; and (ii) a dramatic Tc drop down to ~3 K at a critical pressure of ~9 GPa suggestive of a structural instability. We show that a combined electrical resistivity and x-ray diffraction study under high pressures provides a comprehensive account of both phenomena within the frame of the BCS theory in terms of a P-induced softening of the in-plane Ca mode relevant to the electron–phonon coupling. Our data analysis indicates that, below ~8 GPa, the softening contributes to the Tc enhancement whilst, at higher pressures, it drives the system to a disordered phase presumably characterized by a disordering of the Ca sublattice. Thus, pressure induces a simultaneous order-disorder and lattice-softening phase transition from a good metal phase with high Tc to a bad metal phase with low Tc. More... »

PAGES

407-418

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-90-481-9258-8_33

DOI

http://dx.doi.org/10.1007/978-90-481-9258-8_33

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1000745219


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