Frequencies, times, and forces in the dynamics of Na clusters View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

1999

AUTHORS

P.-G. Reinhard , M. Brack , F. Calvayrac , C. Kohl , S. Kümmel , E. Suraud , C. A. Ullrich

ABSTRACT

Laser excitation of metal clusters depends on various parameters such as frequency, intensity, and pulse time: We give here an overview of relevant time scales and forces for the example of Na clusters. Variation of laser intensity is studied in connection with second harmonic generation. We see a rather sudden transition from a perturbative regime at low intensities to a field-dominated regime for larger intensities. We use the non-linearized time-dependent local density approximation (TDLDA), together with a local pseudopotential for the interaction of the valence electrons with the ions. Explicit ionic motion is taken into account in one test case where we demonstrate the importance of ionic effects for the detailed time evolution at times larger than 100 fs. More... »

PAGES

111-117

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-3-642-88188-6_21

DOI

http://dx.doi.org/10.1007/978-3-642-88188-6_21

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1089714891


Indexing Status Check whether this publication has been indexed by Scopus and Web Of Science using the SN Indexing Status Tool
Incoming Citations Browse incoming citations for this publication using opencitations.net

JSON-LD is the canonical representation for SciGraph data.

TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT

[
  {
    "@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json", 
    "about": [
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/03", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Chemical Sciences", 
        "type": "DefinedTerm"
      }, 
      {
        "id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0306", 
        "inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/", 
        "name": "Physical Chemistry (incl. Structural)", 
        "type": "DefinedTerm"
      }
    ], 
    "author": [
      {
        "affiliation": {
          "alternateName": "Institut f\u00fcr Theoretische Physik, Universit\u00e4t Erlangen, Staudtstrasse 7, D-91058, Erlangen, Germany", 
          "id": "http://www.grid.ac/institutes/grid.5330.5", 
          "name": [
            "Institut f\u00fcr Theoretische Physik, Universit\u00e4t Erlangen, Staudtstrasse 7, D-91058, Erlangen, Germany"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Reinhard", 
        "givenName": "P.-G.", 
        "id": "sg:person.01331316645.49", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01331316645.49"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Theoretical Physics, University of Regensburg, D-93040, Regensburg, Germany", 
          "id": "http://www.grid.ac/institutes/grid.7727.5", 
          "name": [
            "Institute for Theoretical Physics, University of Regensburg, D-93040, Regensburg, Germany"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Brack", 
        "givenName": "M.", 
        "id": "sg:person.012734147145.29", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012734147145.29"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France", 
          "id": "http://www.grid.ac/institutes/grid.15781.3a", 
          "name": [
            "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Calvayrac", 
        "givenName": "F.", 
        "id": "sg:person.013267662541.22", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013267662541.22"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Institute for Nuclear Theory, University of Washington, 98195, Seattle, WA, USA", 
          "id": "http://www.grid.ac/institutes/grid.34477.33", 
          "name": [
            "Institute for Nuclear Theory, University of Washington, 98195, Seattle, WA, USA"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Kohl", 
        "givenName": "C.", 
        "id": "sg:person.010230320662.61", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010230320662.61"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France", 
          "id": "http://www.grid.ac/institutes/grid.15781.3a", 
          "name": [
            "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France"
          ], 
          "type": "Organization"
        }, 
        "familyName": "K\u00fcmmel", 
        "givenName": "S.", 
        "id": "sg:person.0623265245.41", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0623265245.41"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France", 
          "id": "http://www.grid.ac/institutes/grid.15781.3a", 
          "name": [
            "Laboratoire de Physique Quantique, Universit\u00e9 Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Suraud", 
        "givenName": "E.", 
        "id": "sg:person.01112212744.32", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01112212744.32"
        ], 
        "type": "Person"
      }, 
      {
        "affiliation": {
          "alternateName": "Department Of Physics, University of Missouri, 65211, Columbia, MO, USA", 
          "id": "http://www.grid.ac/institutes/grid.134936.a", 
          "name": [
            "Department Of Physics, University of Missouri, 65211, Columbia, MO, USA"
          ], 
          "type": "Organization"
        }, 
        "familyName": "Ullrich", 
        "givenName": "C. A.", 
        "id": "sg:person.01132616124.75", 
        "sameAs": [
          "https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01132616124.75"
        ], 
        "type": "Person"
      }
    ], 
    "datePublished": "1999", 
    "datePublishedReg": "1999-01-01", 
    "description": "Laser excitation of metal clusters depends on various parameters such as frequency, intensity, and pulse time: We give here an overview of relevant time scales and forces for the example of Na clusters. Variation of laser intensity is studied in connection with second harmonic generation. We see a rather sudden transition from a perturbative regime at low intensities to a field-dominated regime for larger intensities. We use the non-linearized time-dependent local density approximation (TDLDA), together with a local pseudopotential for the interaction of the valence electrons with the ions. Explicit ionic motion is taken into account in one test case where we demonstrate the importance of ionic effects for the detailed time evolution at times larger than 100 fs.", 
    "editor": [
      {
        "familyName": "Ch\u00e2telain", 
        "givenName": "A.", 
        "type": "Person"
      }, 
      {
        "familyName": "Bonard", 
        "givenName": "J.-M.", 
        "type": "Person"
      }
    ], 
    "genre": "chapter", 
    "id": "sg:pub.10.1007/978-3-642-88188-6_21", 
    "isAccessibleForFree": false, 
    "isPartOf": {
      "isbn": [
        "978-3-642-88190-9", 
        "978-3-642-88188-6"
      ], 
      "name": "The European Physical Journal D", 
      "type": "Book"
    }, 
    "keywords": [
      "time-dependent local density approximation", 
      "Na clusters", 
      "second harmonic generation", 
      "local density approximation", 
      "laser intensity", 
      "detailed time evolution", 
      "harmonic generation", 
      "laser excitation", 
      "valence electrons", 
      "perturbative regime", 
      "relevant time scales", 
      "ionic motion", 
      "density approximation", 
      "large intensity", 
      "time evolution", 
      "local pseudopotential", 
      "pulse time", 
      "metal clusters", 
      "time scales", 
      "sudden transition", 
      "intensity", 
      "low intensity", 
      "electrons", 
      "regime", 
      "pseudopotentials", 
      "excitation", 
      "ionic effects", 
      "clusters", 
      "ions", 
      "transition", 
      "frequency", 
      "approximation", 
      "motion", 
      "dynamics", 
      "force", 
      "interaction", 
      "evolution", 
      "generation", 
      "parameters", 
      "time", 
      "account", 
      "scale", 
      "test cases", 
      "variation", 
      "effect", 
      "example", 
      "connection", 
      "overview", 
      "cases", 
      "importance"
    ], 
    "name": "Frequencies, times, and forces in the dynamics of Na clusters", 
    "pagination": "111-117", 
    "productId": [
      {
        "name": "dimensions_id", 
        "type": "PropertyValue", 
        "value": [
          "pub.1089714891"
        ]
      }, 
      {
        "name": "doi", 
        "type": "PropertyValue", 
        "value": [
          "10.1007/978-3-642-88188-6_21"
        ]
      }
    ], 
    "publisher": {
      "name": "Springer Nature", 
      "type": "Organisation"
    }, 
    "sameAs": [
      "https://doi.org/10.1007/978-3-642-88188-6_21", 
      "https://app.dimensions.ai/details/publication/pub.1089714891"
    ], 
    "sdDataset": "chapters", 
    "sdDatePublished": "2022-09-02T16:16", 
    "sdLicense": "https://scigraph.springernature.com/explorer/license/", 
    "sdPublisher": {
      "name": "Springer Nature - SN SciGraph project", 
      "type": "Organization"
    }, 
    "sdSource": "s3://com-springernature-scigraph/baseset/20220902/entities/gbq_results/chapter/chapter_456.jsonl", 
    "type": "Chapter", 
    "url": "https://doi.org/10.1007/978-3-642-88188-6_21"
  }
]
 

Download the RDF metadata as:  json-ld nt turtle xml License info

HOW TO GET THIS DATA PROGRAMMATICALLY:

JSON-LD is a popular format for linked data which is fully compatible with JSON.

curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1007/978-3-642-88188-6_21'

N-Triples is a line-based linked data format ideal for batch operations.

curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1007/978-3-642-88188-6_21'

Turtle is a human-readable linked data format.

curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1007/978-3-642-88188-6_21'

RDF/XML is a standard XML format for linked data.

curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1007/978-3-642-88188-6_21'


 

This table displays all metadata directly associated to this object as RDF triples.

168 TRIPLES      22 PREDICATES      75 URIs      68 LITERALS      7 BLANK NODES

Subject Predicate Object
1 sg:pub.10.1007/978-3-642-88188-6_21 schema:about anzsrc-for:03
2 anzsrc-for:0306
3 schema:author N91ebe9a65f2e4aab8bda54f6d7a75639
4 schema:datePublished 1999
5 schema:datePublishedReg 1999-01-01
6 schema:description Laser excitation of metal clusters depends on various parameters such as frequency, intensity, and pulse time: We give here an overview of relevant time scales and forces for the example of Na clusters. Variation of laser intensity is studied in connection with second harmonic generation. We see a rather sudden transition from a perturbative regime at low intensities to a field-dominated regime for larger intensities. We use the non-linearized time-dependent local density approximation (TDLDA), together with a local pseudopotential for the interaction of the valence electrons with the ions. Explicit ionic motion is taken into account in one test case where we demonstrate the importance of ionic effects for the detailed time evolution at times larger than 100 fs.
7 schema:editor Nd8d722b3634c4d21aec36cc9ce703f72
8 schema:genre chapter
9 schema:isAccessibleForFree false
10 schema:isPartOf Ne59261facb0d4cdf998d0ad188b77357
11 schema:keywords Na clusters
12 account
13 approximation
14 cases
15 clusters
16 connection
17 density approximation
18 detailed time evolution
19 dynamics
20 effect
21 electrons
22 evolution
23 example
24 excitation
25 force
26 frequency
27 generation
28 harmonic generation
29 importance
30 intensity
31 interaction
32 ionic effects
33 ionic motion
34 ions
35 large intensity
36 laser excitation
37 laser intensity
38 local density approximation
39 local pseudopotential
40 low intensity
41 metal clusters
42 motion
43 overview
44 parameters
45 perturbative regime
46 pseudopotentials
47 pulse time
48 regime
49 relevant time scales
50 scale
51 second harmonic generation
52 sudden transition
53 test cases
54 time
55 time evolution
56 time scales
57 time-dependent local density approximation
58 transition
59 valence electrons
60 variation
61 schema:name Frequencies, times, and forces in the dynamics of Na clusters
62 schema:pagination 111-117
63 schema:productId N00917dbc69934a5c92bbe5aa2b3a90bc
64 N2179f2aeb7fd48338cddb3be564d47bd
65 schema:publisher N06eb6a5a88f04ebc89ce3fb8fa0dde85
66 schema:sameAs https://app.dimensions.ai/details/publication/pub.1089714891
67 https://doi.org/10.1007/978-3-642-88188-6_21
68 schema:sdDatePublished 2022-09-02T16:16
69 schema:sdLicense https://scigraph.springernature.com/explorer/license/
70 schema:sdPublisher N3ec96ec7c73646f6a183eb3e66288f4e
71 schema:url https://doi.org/10.1007/978-3-642-88188-6_21
72 sgo:license sg:explorer/license/
73 sgo:sdDataset chapters
74 rdf:type schema:Chapter
75 N008b6767f8c245818436377db75bf524 rdf:first Ne32b4918adcc467591670448bcb06d19
76 rdf:rest rdf:nil
77 N00917dbc69934a5c92bbe5aa2b3a90bc schema:name doi
78 schema:value 10.1007/978-3-642-88188-6_21
79 rdf:type schema:PropertyValue
80 N06eb6a5a88f04ebc89ce3fb8fa0dde85 schema:name Springer Nature
81 rdf:type schema:Organisation
82 N124f90f6d60a46ddba007b49d0ffb4bf rdf:first sg:person.013267662541.22
83 rdf:rest Nb126e1eef7ba4fb28cff87e63ac1dd9e
84 N2179f2aeb7fd48338cddb3be564d47bd schema:name dimensions_id
85 schema:value pub.1089714891
86 rdf:type schema:PropertyValue
87 N3ec96ec7c73646f6a183eb3e66288f4e schema:name Springer Nature - SN SciGraph project
88 rdf:type schema:Organization
89 N5ec19f7e7c7149e4bcbe3ec588da2328 rdf:first sg:person.01132616124.75
90 rdf:rest rdf:nil
91 N5f126d39d86a4f9a95cc1359d1543a70 rdf:first sg:person.01112212744.32
92 rdf:rest N5ec19f7e7c7149e4bcbe3ec588da2328
93 N733b58546dfa46c585a802efff1f05b5 schema:familyName Châtelain
94 schema:givenName A.
95 rdf:type schema:Person
96 N7832b5690ed34b30808ed4fc95f35f31 rdf:first sg:person.0623265245.41
97 rdf:rest N5f126d39d86a4f9a95cc1359d1543a70
98 N91ebe9a65f2e4aab8bda54f6d7a75639 rdf:first sg:person.01331316645.49
99 rdf:rest Nc8716a6ca4754addab9b18cfd8dbace3
100 Nb126e1eef7ba4fb28cff87e63ac1dd9e rdf:first sg:person.010230320662.61
101 rdf:rest N7832b5690ed34b30808ed4fc95f35f31
102 Nc8716a6ca4754addab9b18cfd8dbace3 rdf:first sg:person.012734147145.29
103 rdf:rest N124f90f6d60a46ddba007b49d0ffb4bf
104 Nd8d722b3634c4d21aec36cc9ce703f72 rdf:first N733b58546dfa46c585a802efff1f05b5
105 rdf:rest N008b6767f8c245818436377db75bf524
106 Ne32b4918adcc467591670448bcb06d19 schema:familyName Bonard
107 schema:givenName J.-M.
108 rdf:type schema:Person
109 Ne59261facb0d4cdf998d0ad188b77357 schema:isbn 978-3-642-88188-6
110 978-3-642-88190-9
111 schema:name The European Physical Journal D
112 rdf:type schema:Book
113 anzsrc-for:03 schema:inDefinedTermSet anzsrc-for:
114 schema:name Chemical Sciences
115 rdf:type schema:DefinedTerm
116 anzsrc-for:0306 schema:inDefinedTermSet anzsrc-for:
117 schema:name Physical Chemistry (incl. Structural)
118 rdf:type schema:DefinedTerm
119 sg:person.010230320662.61 schema:affiliation grid-institutes:grid.34477.33
120 schema:familyName Kohl
121 schema:givenName C.
122 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.010230320662.61
123 rdf:type schema:Person
124 sg:person.01112212744.32 schema:affiliation grid-institutes:grid.15781.3a
125 schema:familyName Suraud
126 schema:givenName E.
127 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01112212744.32
128 rdf:type schema:Person
129 sg:person.01132616124.75 schema:affiliation grid-institutes:grid.134936.a
130 schema:familyName Ullrich
131 schema:givenName C. A.
132 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01132616124.75
133 rdf:type schema:Person
134 sg:person.012734147145.29 schema:affiliation grid-institutes:grid.7727.5
135 schema:familyName Brack
136 schema:givenName M.
137 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.012734147145.29
138 rdf:type schema:Person
139 sg:person.013267662541.22 schema:affiliation grid-institutes:grid.15781.3a
140 schema:familyName Calvayrac
141 schema:givenName F.
142 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.013267662541.22
143 rdf:type schema:Person
144 sg:person.01331316645.49 schema:affiliation grid-institutes:grid.5330.5
145 schema:familyName Reinhard
146 schema:givenName P.-G.
147 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.01331316645.49
148 rdf:type schema:Person
149 sg:person.0623265245.41 schema:affiliation grid-institutes:grid.15781.3a
150 schema:familyName Kümmel
151 schema:givenName S.
152 schema:sameAs https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.0623265245.41
153 rdf:type schema:Person
154 grid-institutes:grid.134936.a schema:alternateName Department Of Physics, University of Missouri, 65211, Columbia, MO, USA
155 schema:name Department Of Physics, University of Missouri, 65211, Columbia, MO, USA
156 rdf:type schema:Organization
157 grid-institutes:grid.15781.3a schema:alternateName Laboratoire de Physique Quantique, Université Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France
158 schema:name Laboratoire de Physique Quantique, Université Paul Sabatier, 118 Route de Narbonne, F-31062, Toulouse Cedex, France
159 rdf:type schema:Organization
160 grid-institutes:grid.34477.33 schema:alternateName Institute for Nuclear Theory, University of Washington, 98195, Seattle, WA, USA
161 schema:name Institute for Nuclear Theory, University of Washington, 98195, Seattle, WA, USA
162 rdf:type schema:Organization
163 grid-institutes:grid.5330.5 schema:alternateName Institut für Theoretische Physik, Universität Erlangen, Staudtstrasse 7, D-91058, Erlangen, Germany
164 schema:name Institut für Theoretische Physik, Universität Erlangen, Staudtstrasse 7, D-91058, Erlangen, Germany
165 rdf:type schema:Organization
166 grid-institutes:grid.7727.5 schema:alternateName Institute for Theoretical Physics, University of Regensburg, D-93040, Regensburg, Germany
167 schema:name Institute for Theoretical Physics, University of Regensburg, D-93040, Regensburg, Germany
168 rdf:type schema:Organization
 




Preview window. Press ESC to close (or click here)


...