Fe/MCM-41 sylilated catalyst: structural changes determination during the Fischer–Tropsch reaction View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2009

AUTHORS

J. F. Bengoa , N. A. Fellenz , M. V. Cagnoli , L. A. Cano , N. G. Gallegos , A. M. Alvarez , S. G. Marchetti

ABSTRACT

Two Fe/MCM-41 systems, one of them sylilated, were obtained to be used as catalysts in Fischer–Tropsch reaction. They have more than 90% of the iron species located inside the support channels, leading to a narrow crystal size distribution accessible to reactive gases. The samples were characterized by X-ray diffraction, atomic absorption spectroscopy, N2 adsorption, Mössbauer spectroscopy and Fourier transformer infrared spectroscopy. Mössbauer spectroscopy allowed us to demonstrate that the catalytic active species were the same in both catalysts. The only difference between them was the surface hydrophobicity, which decreases the “water gas shift reaction” in the sylilated catalyst. Besides, this solid is more active for hydrocarbon production, with a lower methane yield. More... »

PAGES

5-13

Book

TITLE

LACAME 2008

ISBN

978-3-642-10763-4
978-3-642-10764-1

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-3-642-10764-1_3

DOI

http://dx.doi.org/10.1007/978-3-642-10764-1_3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1045001610


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