Two-Photon Absorption in Near-IR Conjugated Molecules: Design Strategy and Structure–Property Relations View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2010-07-03

AUTHORS

Olga V. Przhonska , Scott Webster , Lazaro A. Padilha , Honghua Hu , Alexey D. Kachkovski , David J. Hagan , Eric W. Van Stryland

ABSTRACT

In the past few years, applications built around two-photon absorption (2PA) have emerged, which require new materials to be designed and characterized in order to discover new applications and to advance the existing ones. This chapter describes the nonlinear optical processes and characterization techniques along with design strategies and structure–property relations of cyanine and cyanine-like molecular structures with the goal of enhancing 2PA in the near-IR for multiphoton fluorescence sensing applications. Specifically, a detailed analysis of the linear and nonlinear optical properties of several classes of polymethine dyes, which include symmetrical and asymmetrical combinations of π-conjugated bridges with electron donating (D) or electron accepting (A) terminal groups, are presented. These structures are: D–π–D, A–π–A, D–π–A, and a quadrupolar type arrangement of D–π–A–π–D. The results of this research combined with the growing literature on structure–property relations in organic materials is moving us closer to the ultimate goal of developing a predictive capability for the nonlinear optical properties of molecules. More... »

PAGES

105-147

References to SciGraph publications

Book

TITLE

Advanced Fluorescence Reporters in Chemistry and Biology I

ISBN

978-3-642-04700-8
978-3-642-04702-2

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-3-642-04702-2_4

DOI

http://dx.doi.org/10.1007/978-3-642-04702-2_4

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1035685427


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