Coordination of U(IV) and U(VI) sulfate hydrate in aqueous solution View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2008

AUTHORS

Christoph Hennig , Satoru Tsushima , Vinzenz Brendler , Atsushi Ikeda , Andreas C. Scheinost , Gert Bernhard

ABSTRACT

Sulfuric acid has been used for in situ leaching of uranium ores at several places, among them Känigstein/Germany. The fate of the remaining leaching solvents may pose a substantial problem when released into aquifers used for drinking water. The current available thermodynamic data on uranium sulfate species in aqueous solution are not sufficient because typical leaching solutions commonly exceed the limit of ionic strengths of conventional models. The application of spectroscopic techniques may help to provide the missing data. We review here coordination data of U(IV) and U(VI) sulfate in aqueous solutions with high ionic strengths investigated by several spectroscopic techniques (mainly EXAFS) combined with XRD studies and DFT calculations. The observed results expand the current knowledge of uranium sulfates substantially beyond the available information based mainly on thermodynamic data. More... »

PAGES

603-614

Book

TITLE

Uranium, Mining and Hydrogeology

ISBN

978-3-540-87745-5
978-3-540-87746-2

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-3-540-87746-2_75

DOI

http://dx.doi.org/10.1007/978-3-540-87746-2_75

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1043117483


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