Can We Explain the Observed Decrease in Secondary Inorganic Aerosol and Its Precursors Between 1990 and 2009 over Europe Using ... View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2014-03-28

AUTHORS

S. Banzhaf , M. Schaap , R. Kranenburg , A. M. M. Manders , A. J. Segers , A. H. J. Visschedijk , H. A. C. Denier van der Gon , J. J. P. Kuenen , C. Hendriks , E. van Meijgaard , L. H. van Ulft , P. J. H. Builtjes

ABSTRACT

In this study we investigate the ability of the Chemistry Transport Model (CTM) LOTOS-EUROS to explain the observed decrease in secondary inorganic aerosol (SIA) and its precursors between 1990 and 2009 over Europe. The model explicitly accounts for cloud chemistry and aerosol thermodynamics. The results have shown that the model largely captures the observed trends in SIA and its precursors’ concentrations while it underestimates the interannual variability. Using a source-apportionment module the amount of SIA formed per unit emission was traced for a number of regions. The results show 20–50 % more efficient SO42− formation in 2009 compared to 1990, whereas the change in NO3− formation per unit NOx emission is lower (−10 % to +20 %) for the same time period. More... »

PAGES

481-488

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/978-3-319-04379-1_79

DOI

http://dx.doi.org/10.1007/978-3-319-04379-1_79

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1028622032


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