Effect of Boundary Condition Fluctuations on Smoluchowski Reaction Rates View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2001-01-23

AUTHORS

Charles R. Doering

ABSTRACT

We formulate, solve, and examine an elementary model of gated absorption, where the reactivity of a sphere fluctuates in time, in the context of Smolukowski’s diffusion-controlled rate processes. Interest in this problem was stimulated by some experiments on biomolecular rate processes in the 1970s. The model under discussion here was studied by a number of investigators in the 1980s, and interest is renewed by the discovery of resonant activation in the 1990s. We find that the simplest gated reaction process does not exhibit features characteristic of resonant activation, although some interesting nonequilibrium correlations may have a quantitative effect in some situations. We speculate on the possible appearance of resonant activation phenomena in related processes. More... »

PAGES

316-326

References to SciGraph publications

Book

TITLE

Stochastic Processes in Physics, Chemistry, and Biology

ISBN

978-3-540-41074-4

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/3-540-45396-2_29

DOI

http://dx.doi.org/10.1007/3-540-45396-2_29

DIMENSIONS

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131 https://www.grid.ac/institutes/grid.214458.e schema:alternateName University of Michigan–Ann Arbor
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