Photoiniferter-Driven Precision Surface Graft Microarchitectures for Biomedical Applications View Full Text


Ontology type: schema:Chapter     


Chapter Info

DATE

2006

AUTHORS

Takehisa Matsuda

ABSTRACT

The photoiniferter polymerization method proposed by Otsu et al. was utilized to generate well-controlled graft polymer chains on a surface. The “livingness” of graft chains, coupled with the inherent nature of photochemical processing, enables the development of complex graft-polymerized surface designs with controlled graft-chain length and composition, regiospecific addressability and high-dimensional precision. As an extension of the advantageous features of the “quasi-living” nature of polymerization, precise control technology for surface graft-chain architectures, which show multibranching, a fractal hierarchy and a gradient segmental density, was elaborated. The logical programmed morphogenesis approach was discussed, and a high degree of graft-chain architectures was demonstrated as if these resemble the spatiogeometric analogue models of growing trees with diverse morphologies. The confocal laser scanning microscopic measurement for dye-stained grafted surfaces and the force–distance curves of atomic force microscopy provided some physicochemical and structural insights into graft architectures. Under appropriate conditions, the cross-recommendation reaction of two different dithiocarbamate derivatives enabled the development of a novel surface derivatization method. Microprocessed surfaces with multigraft polymers in different regions and with different chain lengths enabled differentiation of regiospecific cell adhesion and proliferation potentials and cellular functions in one sample, which provides high-throughput screening for the biocompatibility of designed medical devices. More... »

PAGES

67-106

References to SciGraph publications

  • 1990-05. Preparation of Phospholipid Polylners and Their Properties as Polymer Hydrogel Membranes in POLYMER JOURNAL
  • 1999-05-27. Controlled Synthesis of Polymers Using the Iniferter Technique: Developments in Living Radical Polymerization in MICROENCAPSULATION MICROGELS INIFERTERS
  • 1985. Polymer Surface Dynamics in SURFACE AND INTERFACIAL ASPECTS OF BIOMEDICAL POLYMERS
  • Book

    TITLE

    Surface-Initiated Polymerization I

    ISBN

    978-3-540-30247-6
    978-3-540-33392-0

    Author Affiliations

    Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1007/12_065

    DOI

    http://dx.doi.org/10.1007/12_065

    DIMENSIONS

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